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    Structure of polydisperse inverse ferrofluids: Theory and computer simulation

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    Genre
    Journal Article
    Date
    2008-01-24
    Author
    Jian, YC
    Gao, Y
    Huang, JP
    Tao, R
    Subject
    Colloids
    Computer Simulation
    Ferric Compounds
    Magnetics
    Metal Nanoparticles
    Models, Molecular
    Particle Size
    Thermodynamics
    Permanent link to this record
    http://hdl.handle.net/20.500.12613/6093
    
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    DOI
    10.1021/jp075849h
    Abstract
    By using theoretical analysis and molecular dynamics simulations, we investigate the structure of colloidal crystals formed by nonmagnetic microparticles (or magnetic holes) suspended in ferrofluids (called inverse ferrofluids), by taking into account the effect of polydispersity in size of the nonmagnetic microparticles. Such polydispersity often exists in real situations. We obtain an analytical expression for the interaction energy of monodisperse, bidisperse, and polydisperse inverse ferrofluids. Body-centered tetragonal (bet) lattices are shown to possess the lowest energy when compared with other sorts of lattices and thus serve as the ground state of the systems. Also, the effect of microparticle size distributions (namely, polydispersity in size) plays an important role in the formation of various kinds of structural configurations. Thus, it seems possible to fabricate colloidal crystals by choosing appropriate polydispersity in size. © 2008 American Chemical Society.
    Citation to related work
    American Chemical Society (ACS)
    Has part
    Journal of Physical Chemistry B
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    ae974a485f413a2113503eed53cd6c53
    http://dx.doi.org/10.34944/dspace/6075
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