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    Molecular-ion trap-depletion spectroscopy of BaCl<sup>+</sup>

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    Genre
    Journal Article
    Date
    2011-03-09
    Author
    Chen, K
    Schowalter, SJ
    Kotochigova, S
    Petrov, A
    Rellergert, WG
    Sullivan, ST
    Hudson, ER
    Subject
    physics.atom-ph
    physics.atom-ph
    physics.chem-ph
    Permanent link to this record
    http://hdl.handle.net/20.500.12613/6043
    
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    DOI
    10.1103/PhysRevA.83.030501
    Abstract
    We demonstrate a simple technique for molecular-ion spectroscopy. BaCl + molecular ions are trapped in a linear Paul trap in the presence of a room-temperature He buffer gas and photodissociated by driving an electronic transition from the ground X 1Σ+ state to the repulsive wall of the A 1Π state. The photodissociation spectrum is recorded by monitoring the induced trap loss of BaCl+ ions as a function of excitation wavelength. Accurate molecular potentials and spectroscopic constants are determined. A comparison of the theoretical photodissociation cross sections with the measurements shows excellent agreement. This study represents an important step toward the production of ultracold ground-state molecular ions. © 2011 American Physical Society.
    Citation to related work
    American Physical Society (APS)
    Has part
    Physical Review A - Atomic, Molecular, and Optical Physics
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    ae974a485f413a2113503eed53cd6c53
    http://dx.doi.org/10.34944/dspace/6025
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