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    Trapping molecular ions formed via photo-associative ionization of ultracold atoms

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    Genre
    Journal Article
    Date
    2011-11-14
    Author
    Sullivan, ST
    Rellergert, WG
    Kotochigova, S
    Chen, K
    Schowalter, SJ
    Hudson, ER
    Subject
    physics.atom-ph
    physics.atom-ph
    physics.chem-ph
    Permanent link to this record
    http://hdl.handle.net/20.500.12613/6019
    
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    DOI
    10.1039/c1cp21205b
    Abstract
    The formation of 40Ca2+ molecular ions is observed in a hybrid 40Ca magneto-optical and ion trap system. The molecular ion formation process is determined to be photo-associative ionization of ultracold 40Ca atoms. A lower bound for the two-body rate constant is found to be ≥ 2 ± 1 × 10-15 cm 3 Hz. Ab initio molecular potential curves are calculated for the neutral Ca2 and ionic Ca2+ molecules and used in a model that identifies the photo-associative ionization pathway. As this technique does not require a separate photo-association laser, it could find use as a simple, robust method for producing ultracold molecular ions. © the Owner Societies 2011.
    Citation to related work
    Royal Society of Chemistry (RSC)
    Has part
    Physical Chemistry Chemical Physics
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    http://dx.doi.org/10.34944/dspace/6001
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