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    Momentum-resolved electronic structure at a buried interface from soft X-ray standing-wave angle-resolved photoemission

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    Genre
    Journal Article
    Date
    2013-10-01
    Author
    Gray, AX
    Minár, J
    Plucinski, L
    Huijben, M
    Bostwick, A
    Rotenberg, E
    Yang, SH
    Braun, J
    Winkelmann, A
    Conti, G
    Eiteneer, D
    Rattanachata, A
    Greer, AA
    Ciston, J
    Ophus, C
    Rijnders, G
    Blank, DHA
    Doennig, D
    Pentcheva, R
    Kortright, JB
    Schneider, CM
    Ebert, H
    Fadley, CS
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    Subject
    cond-mat.mtrl-sci
    cond-mat.mtrl-sci
    Permanent link to this record
    http://hdl.handle.net/20.500.12613/5936
    
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    DOI
    10.1209/0295-5075/104/17004
    Abstract
    Angle-resolved photoemission spectroscopy (ARPES) is a powerful technique for the study of electronic structure, but it lacks a direct ability to study buried interfaces between two materials. We address this limitation by combining ARPES with soft X-ray standing-wave (SW) excitation (SWARPES), in which the SW profile is scanned through the depth of the sample. We have studied the buried interface in a prototypical magnetic tunnel junction La0.7Sr 0.3MnO3/SrTiO3. Depth-and momentum-resolved maps of Mn 3d eg and t2g states from the central, bulk-like and interface-like regions of La0.7Sr0.3MnO 3 exhibit distinctly different behavior consistent with a change in the Mn bonding at the interface. We compare the experimental results to state-of-the-art density-functional and one-step photoemission theory, with encouraging agreement that suggests wide future applications of this technique. © Copyright EPLA, 2013.
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    ae974a485f413a2113503eed53cd6c53
    http://dx.doi.org/10.34944/dspace/5918
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