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    Measurement of collective excitations in VO2 by resonant inelastic x-ray scattering

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    1603.01164v1.pdf
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    Genre
    Pre-print
    Date
    2016-10-21
    Author
    He, H
    Gray, AX
    Granitzka, P
    Jeong, JW
    Aetukuri, NP
    Kukreja, R
    Miao, L
    Breitweiser, SA
    Wu, J
    Huang, YB
    Olalde-Velasco, P
    Pelliciari, J
    Schlotter, WF
    Arenholz, E
    Schmitt, T
    Samant, MG
    Parkin, SSP
    Dürr, HA
    Wray, LA
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    Subject
    cond-mat.str-el
    cond-mat.str-el
    Permanent link to this record
    http://hdl.handle.net/20.500.12613/5002
    
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    DOI
    10.1103/PhysRevB.94.161119
    Abstract
    © 2016 American Physical Society. Vanadium dioxide is of broad interest as a spin-12 electron system that realizes a metal-insulator transition near room temperature, due to a combination of strongly correlated and itinerant electron physics. Here, resonant inelastic x-ray scattering is used to measure the excitation spectrum of charge and spin degrees of freedom at the vanadium L edge under different polarization and temperature conditions, revealing excitations that differ greatly from those seen in optical measurements. These spectra encode the evolution of short-range energetics across the metal-insulator transition, including the low-temperature appearance of a strong candidate for the singlet-triplet excitation of a vanadium dimer.
    Citation to related work
    American Physical Society (APS)
    Has part
    Physical Review B
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    ae974a485f413a2113503eed53cd6c53
    http://dx.doi.org/10.34944/dspace/4984
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