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dc.creatorYang, X
dc.creatorTong, H
dc.creatorWang, WH
dc.creatorChen, K
dc.date.accessioned2020-12-11T16:12:35Z
dc.date.available2020-12-11T16:12:35Z
dc.date.issued2019-06-28
dc.identifier.issn2470-0045
dc.identifier.issn2470-0053
dc.identifier.doihttp://dx.doi.org/10.34944/dspace/4303
dc.identifier.other31330594 (pubmed)
dc.identifier.urihttp://hdl.handle.net/20.500.12613/4321
dc.description.abstract© 2019 American Physical Society. Using video microscopy, we measure local spatial constraints in disordered binary colloidal samples, ranging from dilute fluids to jammed glasses, and probe their spatial and temporal correlations to local dynamics during the glass transition. We observe the emergence of significant correlations between constraints and local dynamics within the Lindemann criterion, which coincides with the onset of glassy dynamics in supercooled liquids. Rigid domains in fluids are identified based on local constraints and demonstrate a percolation transition near the glass transition, accompanied by the emergence of dynamical heterogeneities. Our results show that spatial constraint instead of the geometry of amorphous structures is the key that connects the complex spatial-temporal correlations in disordered materials.
dc.format.extent062610-
dc.language.isoen
dc.relation.haspartPhysical Review E
dc.relation.isreferencedbyAmerican Physical Society (APS)
dc.rightsAll Rights Reserved
dc.subjectcond-mat.soft
dc.subjectcond-mat.soft
dc.subjectcond-mat.dis-nn
dc.subjectcond-mat.mtrl-sci
dc.subjectcond-mat.stat-mech
dc.titleEmergence and percolation of rigid domains during the colloidal glass transition
dc.typeArticle
dc.type.genrePre-print
dc.relation.doi10.1103/PhysRevE.99.062610
dc.ada.noteFor Americans with Disabilities Act (ADA) accommodation, including help with reading this content, please contact scholarshare@temple.edu
dc.date.updated2020-12-11T16:12:32Z
refterms.dateFOA2020-12-11T16:12:35Z


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